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Magnetoresistivity of hydrogen-doped Zr2(3d) metallic glasses

Identifieur interne : 000925 ( Main/Repository ); précédent : 000924; suivant : 000926

Magnetoresistivity of hydrogen-doped Zr2(3d) metallic glasses

Auteurs : RBID : Pascal:13-0304828

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English descriptors

Abstract

Magnetoresistivity of (Zr2(3d))1 - xHx metallic glasses (where 3d stands for Fe and Co atoms) was investigated as a function of hydrogen doping (x) in the temperature range from 100 K down to 5 K. Obtained magnetoresistivity is always positive due to the strong spin-orbit interaction and well described in the terms of exchange-enhanced spin-splitting contributions to the usual weak-localization term. (Zr2Fe)1 - xHx exhibits a significantly stronger magnetoresistivity than (Zr2Co)1 - xHx for all measured temperatures and doping levels, which is attributed to the increase in the inelastic spin-scattering rate (τ-1in) and the Stoner factor (1 - I)-1. The magnetoresistivity of (Zr2(3d))1 - xHx exhibits a simple B2 behavior at higher temperatures, providing the information on τ-1in, and a more complex behavior at low temperatures, which gives the information on the spin-orbit scattering rate (τ-1so). It was found that the increase in the doping level reduces τ-1so, indicating hybridization of hydrogen s-electrons with Zr d-electrons and thus reducing the spin-orbit interaction.

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Pascal:13-0304828

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<title xml:lang="en" level="a">Magnetoresistivity of hydrogen-doped Zr
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(3d) metallic glasses</title>
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<name sortKey="Novak, M" uniqKey="Novak M">M. Novak</name>
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<s1>Department of Physics, Faculty of Science, University of Zagreb, Bijeniˇcka cesta 32</s1>
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<sZ>1 aut.</sZ>
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<name sortKey="Kokanovic, I" uniqKey="Kokanovic I">I. Kokanovic</name>
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<s1>Department of Physics, Faculty of Science, University of Zagreb, Bijeniˇcka cesta 32</s1>
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<idno type="ISSN">0022-3093</idno>
<title level="j" type="abbreviated">J. non-cryst. solids</title>
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<term>Hybridization</term>
<term>Indium additions</term>
<term>Inelastic scattering</term>
<term>Magnetoresistance</term>
<term>Metallic glasses</term>
<term>Spin exchange</term>
<term>Spin fluctuations</term>
<term>Spin-orbit interactions</term>
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<term>Dopage</term>
<term>Addition indium</term>
<term>Dépendance température</term>
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<term>Interaction spin orbite</term>
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<term>Interaction échange</term>
<term>Echange spin</term>
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<div type="abstract" xml:lang="en">Magnetoresistivity of (Zr
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(3d))
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<sub>-</sub>
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H
<sub>x</sub>
metallic glasses (where 3d stands for Fe and Co atoms) was investigated as a function of hydrogen doping (x) in the temperature range from 100 K down to 5 K. Obtained magnetoresistivity is always positive due to the strong spin-orbit interaction and well described in the terms of exchange-enhanced spin-splitting contributions to the usual weak-localization term. (Zr
<sub>2</sub>
Fe)
<sub>1</sub>
<sub>-</sub>
<sub>x</sub>
H
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exhibits a significantly stronger magnetoresistivity than (Zr
<sub>2</sub>
Co)
<sub>1</sub>
<sub>-</sub>
<sub>x</sub>
H
<sub>x</sub>
for all measured temperatures and doping levels, which is attributed to the increase in the inelastic spin-scattering rate (τ
<sup>-1</sup>
<sub>in</sub>
) and the Stoner factor (1 - I)
<sup>-1</sup>
. The magnetoresistivity of (Zr
<sub>2</sub>
(3d))
<sub>1</sub>
<sub>-</sub>
<sub>x</sub>
H
<sub>x</sub>
exhibits a simple B
<sup>2</sup>
behavior at higher temperatures, providing the information on τ
<sup>-1</sup>
<sub>in</sub>
, and a more complex behavior at low temperatures, which gives the information on the spin-orbit scattering rate (τ
<sup>-1</sup>
<sub>so</sub>
). It was found that the increase in the doping level reduces τ
<sup>-1</sup>
<sub>so</sub>
, indicating hybridization of hydrogen s-electrons with Zr d-electrons and thus reducing the spin-orbit interaction.</div>
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<sub>-</sub>
<sub>x</sub>
H
<sub>x</sub>
metallic glasses (where 3d stands for Fe and Co atoms) was investigated as a function of hydrogen doping (x) in the temperature range from 100 K down to 5 K. Obtained magnetoresistivity is always positive due to the strong spin-orbit interaction and well described in the terms of exchange-enhanced spin-splitting contributions to the usual weak-localization term. (Zr
<sub>2</sub>
Fe)
<sub>1</sub>
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<sub>2</sub>
Co)
<sub>1</sub>
<sub>-</sub>
<sub>x</sub>
H
<sub>x</sub>
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<sup>-1</sup>
<sub>in</sub>
) and the Stoner factor (1 - I)
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. The magnetoresistivity of (Zr
<sub>2</sub>
(3d))
<sub>1</sub>
<sub>-</sub>
<sub>x</sub>
H
<sub>x</sub>
exhibits a simple B
<sup>2</sup>
behavior at higher temperatures, providing the information on τ
<sup>-1</sup>
<sub>in</sub>
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<sup>-1</sup>
<sub>so</sub>
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<sup>-1</sup>
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